Easily the most interesting store we saw this last time in New York was Brooklyn's CB I Hate Perfume. The perfume gallery and laboratory of perfumer Christopher Brosius displays a series of fascinating accords (single scents like blood orange or dandelion) and perfumes (blends of various accords). Naturally you'll need to visit for full effect but his fragrances are available for purchase online and many of the perfumes are also sold in small sizes.
Start with these and if you like them you can come in for a consultation to blend your very own custom perfume! It's not cheap (anywhere from $125-400 depending on the complexity of your formulation) but doesn't cost as much as you would think considering you're getting a one-of-a-kind fragrance.
Go to the store's website for more information.
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